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Journal Articles

Thinning behavior of solid boron carbide immersed in molten stainless steel for core disruptive accident of sodium-cooled fast reactor

Emura, Yuki; Takai, Toshihide; Kikuchi, Shin; Kamiyama, Kenji; Yamano, Hidemasa; Yokoyama, Hiroki*; Sakamoto, Kan*

Journal of Nuclear Science and Technology, 10 Pages, 2023/00

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

Journal Articles

Determination of site occupancy of boron in 6H-SiC by multiple-wavelength neutron holography

Hayashi, Koichi*; Lederer, M.*; Fukumoto, Yohei*; Goto, Masashi*; Yamamoto, Yuta*; Happo, Naohisa*; Harada, Masahide; Inamura, Yasuhiro; Oikawa, Kenichi; Oyama, Kenji*; et al.

Applied Physics Letters, 120(13), p.132101_1 - 132101_6, 2022/03

 Times Cited Count:0 Percentile:0(Physics, Applied)

Journal Articles

Design of a portable backup shutdown system for the high temperature gas cooled reactor

Hamamoto, Shimpei; Ho, H. Q.; Iigaki, Kazuhiko; Goto, Minoru; Shimazaki, Yosuke; Sawahata, Hiroaki; Ishitsuka, Etsuo

Nuclear Engineering and Design, 386, p.111564_1 - 111564_8, 2022/01

 Times Cited Count:1 Percentile:31.61(Nuclear Science & Technology)

The experience of Fukushima Daiichi Nuclear Power Plant accident caused by the great earthquake that occurred in eastern Japan in 2011 showed the importance of preparing for the loss of function of the engineered safety features. Increasing the strength of equipment to prevent loss of function in an accident is effective, but the possibility of loss of function remains. Therefore, it is important to have an alternative to lost functions in order to put the accident under control early. Thus, this study designed an alternative shutdown system, namely a portable backup shutdown system (PBSS), to make countermeasures in the event of a loss of shutdown function more robust without impairing economic efficiency of the High Temperature Gas-cooled Reactor (HTGR). The PBSS is portable and capable of being installed manually so that it can operate in a total loss of off-site electricity. Various neutron absorber materials for the PBSS were also considered from the viewpoints of technical and cost-effective properties. As results of optimization, the boron nitride (BN) was selected as it shows a good neutronic property as well as a reasonable cost in comparison with other materials.

Journal Articles

Thermophysical properties of austenitic stainless steel containing boron carbide in a solid state

Takai, Toshihide; Furukawa, Tomohiro; Yamano, Hidemasa

Mechanical Engineering Journal (Internet), 8(4), p.20-00540_1 - 20-00540_11, 2021/08

In a core disruptive accident scenario, boron carbide, which is used as a control rod material, may melt below the melting temperature of stainless steel owing to the eutectic reaction with them. The eutectic mixture produced is assumed to extensively relocate in the degraded core, and this behavior plays an important role in significantly reducing the neutronic reactivity. However, these behaviors have never been simulated in previous severe accident analysis. To contribute to the improvement of the core disruptive accident analysis code, the thermophysical properties of the eutectic mixture in the solid state were measured, and regression equations that show the temperature (and boron carbide concentration) dependence are created.

Journal Articles

Visualization of the boron distribution in core material melting and relocation specimen by neutron energy resolving method

Abe, Yuta; Tsuchikawa, Yusuke; Kai, Tetsuya; Matsumoto, Yoshihiro*; Parker, J. D.*; Shinohara, Takenao; Oishi, Yuji*; Kamiyama, Takashi*; Nagae, Yuji; Sato, Ikken

JPS Conference Proceedings (Internet), 33, p.011075_1 - 011075_6, 2021/03

Journal Articles

Study of charged particle activation analysis, 2; Determination of boron concentration in human blood samples

Ikebe, Yurie*; Oshima, Masumi*; Bamba, Shigeru*; Asai, Masato; Tsukada, Kazuaki; Sato, Tetsuya; Toyoshima, Atsushi*; Bi, C.*; Seto, Hirofumi*; Amano, Hikaru*; et al.

Applied Radiation and Isotopes, 164, p.109106_1 - 109106_7, 2020/10

 Times Cited Count:2 Percentile:24.28(Chemistry, Inorganic & Nuclear)

Boron Neutron Capture Therapy (BNCT) is a radiotherapy for the treatment of intractable cancer. In BNCT precise determination of $$^{10}$$B concentration in whole blood sample before neutron irradiation is crucial for control of the neutron irradiation time and the neutron dosimetry. We have applied the Charged Particle Activation Analysis (CPAA) to non-destructive and accurate determination of $$^{10}$$B concentration in whole blood sample. The experiment was performed at JAEA Tandem Accelerator using an 8 MeV proton beam. The 478 keV $$gamma$$ ray of $$^{7}$$Be produced in the $$^{10}$$B(p,$$alpha$$)$$^{7}$$Be reaction was used to quantify the $$^{10}$$B, and $$gamma$$ rays of $$^{56}$$Co originating from the reaction with Fe in blood was used to normalize the $$gamma$$-ray intensity. The results demonstrated that the present CPAA method can be applied to the determination of the $$^{10}$$B concentration in the blood sample.

Journal Articles

Journal Articles

Development of three-dimensional distribution visualization technology for boron using energy resolved neutron-imaging system (RADEN)

Abe, Yuta; Tsuchikawa, Yusuke; Kai, Tetsuya; Matsumoto, Yoshihiro*; Parker, J. D.*; Shinohara, Takenao; Oishi, Yuji*; Kamiyama, Takashi*; Nagae, Yuji; Sato, Ikken

Proceedings of 2020 International Conference on Nuclear Engineering (ICONE 2020) (Internet), 6 Pages, 2020/08

Journal Articles

Preparation, thermoelectric properties, and crystal structure of boron-doped Mg$$_{2}$$Si single crystals

Hayashi, Kei*; Saito, Wataru*; Sugimoto, Kazuya*; Oyama, Kenji*; Hayashi, Koichi*; Happo, Naohisa*; Harada, Masahide; Oikawa, Kenichi; Inamura, Yasuhiro; Miyazaki, Yuzuru*

AIP Advances (Internet), 10(3), p.035115_1 - 035115_7, 2020/03

 Times Cited Count:16 Percentile:73.04(Nanoscience & Nanotechnology)

Journal Articles

Boron chemistry during transportation in the high temperature region of a boiling water reactor under severe accident conditions

Miwa, Shuhei; Takase, Gaku; Imoto, Jumpei; Nishioka, Shunichiro; Miyahara, Naoya; Osaka, Masahiko

Journal of Nuclear Science and Technology, 57(3), p.291 - 300, 2020/03

 Times Cited Count:7 Percentile:55.67(Nuclear Science & Technology)

For the evaluation of transport behavior of control material boron in a severe accident of BWR from the viewpoint of chemical effects on cesium and iodine behavior, boron chemistry during transportation in the high temperature region above 400 K was experimentally investigated. The heating tests of boron oxide specimen were conducted using the dedicated experimental apparatus reproducing fission product release and transport in steam atmosphere. Released boron oxide vapor was deposited above 1,000 K by the condensation onto stainless steel. The boron deposits and/or vapors significantly reacted with stainless steel above 1,000 K and formed the stable iron-boron mixed oxide (FeO)$$_{2}$$BO$$_{3}$$. These results indicate that released boron from degraded BWR control blade in a severe accident could remain in the high temperature region such as a Reactor Pressure Vessel. Based on these results, it can be said that the existence of boron deposits in the high temperature region would decrease the amount of transported cesium vapors from a Reactor Pressure Vessel due to possible formation of low volatile cesium borate compounds by the reaction of boron deposits with cesium vapors.

Journal Articles

Thermophysical properties of stainless steel containing 5 mass%B$$_{4}$$C in the solid phase

Takai, Toshihide; Furukawa, Tomohiro; Yamano, Hidemasa

Nuclear Technology, 205(9), p.1164 - 1174, 2019/09

 Times Cited Count:7 Percentile:61.94(Nuclear Science & Technology)

Journal Articles

Study on eutectic melting behavior of control rod materials in core disruptive accidents of sodium-cooled fast reactor, 2; Effect of B$$_{4}$$C addition on thermophysical properties of austenitic stainless steel in a solid state

Takai, Toshihide; Furukawa, Tomohiro; Yamano, Hidemasa

Proceedings of International Nuclear Fuel Cycle Conference / Light Water Reactor Fuel Performance Conference (Global/Top Fuel 2019) (USB Flash Drive), p.847 - 852, 2019/09

Journal Articles

Chemical reaction kinetics dataset of Cs-I-B-Mo-O-H system for evaluation of fission product chemistry under LWR severe accident conditions

Miyahara, Naoya; Miwa, Shuhei; Horiguchi, Naoki; Sato, Isamu*; Osaka, Masahiko

Journal of Nuclear Science and Technology, 56(2), p.228 - 240, 2019/02

 Times Cited Count:7 Percentile:61.94(Nuclear Science & Technology)

In order to improve LWR source term under severe accident conditions, the first version of a fission product (FP) chemistry database named "ECUME" was developed. The ECUME is intended to include major chemical reactions and their effective kinetic constants for representative SA sequences. It is expected that the ECUME can serve as a fundamental basis from which FP chemical models in the SA analysis codes can be elaborated. The implemented chemical reactions in the first version were those for representative gas species in Cs-I-B-Mo-O-H system. The chemical reaction kinetic constants were evaluated from either literature data or calculated values using ab-initio calculations. The sample chemical reaction calculation using the presently constructed dataset showed meaningful kinetics effects at 1000 K. Comparison of the chemical equilibrium compositions by using the dataset with those by chemical equilibrium calculations has shown rather good consistency for the representative Cs-I-B-Mo-O-H species. From these results, it was concluded that the present dataset should be useful to evaluate FP chemistry in Cs-I-B-Mo-O-H system under LWA SA conditions.

Journal Articles

Retention of uranium in cement systems; Effects of cement degradation and complexing ligands

Ochs, M.*; Vriens, B.*; Tachi, Yukio

Progress in Nuclear Science and Technology (Internet), 5, p.208 - 212, 2018/11

The clean-up activities related to the accident at the Fukushima Nuclear Power Plant give rise to several types of wastes containing cementitious materials, such as concrete. Further, the use of cement-based barriers may be considered, due to their favorable and stable chemical properties, including their ability to sorb or incorporate radionuclides. Wastes from Fukushima are expected to contain substances that can have perturbing effects on retention, especially organic complexing substances, boron, and chloride salts. The present study focuses on a methodology for quantifying the retention behaviour of UVI) and U(IV) in cement materials of different degradation and in the presence of organics, boron, and salts on the basis of available literature information. A stepwise approach is proposed and illustrated for Kd setting for U(VI) and U(IV).

Journal Articles

Thermophysical properties of stainless steel containing 5mass%-B$$_{4}$$C in the solid phase

Takai, Toshihide; Furukawa, Tomohiro; Yamano, Hidemasa

Proceedings of 2018 International Congress on Advances in Nuclear Power Plants (ICAPP 2018) (CD-ROM), p.1007 - 1013, 2018/04

Journal Articles

Prediction of chemical effects of Mo and B on the Cs chemisorption onto stainless steel

Di Lemma, F. G.; Yamashita, Shinichiro; Miwa, Shuhei; Nakajima, Kunihisa; Osaka, Masahiko

Energy Procedia, 127, p.29 - 34, 2017/09

 Times Cited Count:4 Percentile:90.81(Energy & Fuels)

Chemical effects of molybdenum (Mo) and boron (B), which were considered to form compounds with Cs, on the Cs chemisorption were predicted using a chemical equilibrium calculation. It is seen that Cs$$_{2}$$MoO$$_{4}$$ were formed in the chemisorbed compounds. On the other hand, little effects were observed for B. The results suggest that the effects of Mo should be considered for further experimental investigation.

Journal Articles

Examination of $$^{131}$$I and $$^{137}$$Cs releases during late phase of Fukushima Daiichi NPP accident by using $$^{131}$$I/$$^{137}$$Cs ratio of source terms evaluated reversely by WSPEEDI code with environmental monitoring data

Hidaka, Akihide; Yokoyama, Hiroya

Journal of Nuclear Science and Technology, 54(8), p.819 - 829, 2017/08

AA2016-0500.pdf:0.44MB

 Times Cited Count:12 Percentile:75.51(Nuclear Science & Technology)

To clarify what happened during the Fukushima accident, the phenomena within RPV and the discussion of ties with the environmental monitoring are very important. However, the previous study has not necessarily advanced until the present that passed almost six years from the accident. The present study investigated $$^{131}$$I and $$^{137}$$Cs release behaviors during the late phase of the accident based on $$^{131}$$I/$$^{137}$$Cs ratio of the source terms that were recently evaluated backward by WSPEEDI code based on environmental monitoring data. The $$^{131}$$I release from the contaminated water in the basement of 1F2 and 1F3 reactor buildings was evaluated to be about 10% of $$^{131}$$I source term. The increase in $$^{137}$$Cs release from March 21 to 23 and from March 30 to 31 could be explained by the release of CsBO$$_{2}$$ which is formed as a result of chemical reactions of Cs with B$$_{4}$$C due to re-ascension of the core temperature caused by slight shortage of the core cooling water.

Journal Articles

Basic visualization experiments on eutectic reaction between boron carbide and stainless steel under sodium-cooled fast reactor conditions

Yamano, Hidemasa; Suzuki, Toru; Kamiyama, Kenji; Kudo, Isamu*

Proceedings of International Conference on Fast Reactors and Related Fuel Cycles; Next Generation Nuclear Systems for Sustainable Development (FR-17) (USB Flash Drive), 11 Pages, 2017/06

This paper describes basic visualization experiments on eutectic reaction and relocation of boron carbide (B$$_{4}$$C) and stainless steel (SS) under a high temperature condition exceeding 1500$$^{circ}$$C as well as the importance of such behaviors in molten core during a core disruptive accident in a Generation-IV sodium-cooled fast reactor (750 MWe class) designed in Japan. At first, a reactivity history was calculated using an exact perturbation calculation tool taking into account expected behaviors. This calculation indicated the importance of a relocation behavior of the B$$_{4}$$C-SS eutectic because its behavior has a large uncertainty in the reactivity history. To clarify this behavior, basic experiments were carried out by visualizing the reaction of a B$$_{4}$$C pellet contacted with molten SS in a high temperature-heating furnace. The experiments have shown the eutectic reaction visualization as well as freezing and relocation of the B$$_{4}$$C-SS eutectic in upper part of the solidified test piece due to the density separation.

Journal Articles

Study on the distribution of boron in the in-vessel fuel debris in conditions close to Fukushima Daiichi Nuclear Power Station Unit 2

Ikeuchi, Hirotomo; Piluso, P.*; Fouquart, P.*; Excoffier, E.*; David, C.*; Brackx, E.*

Proceedings of 8th European Review Meeting on Severe Accident Research (ERMSAR 2017) (Internet), 12 Pages, 2017/05

no abstracts in English

105 (Records 1-20 displayed on this page)